77 research outputs found
Dimensionality-driven spin-flop transition in quasi-one-dimensional PrBa2Cu4O8
In the quasi-one-dimensional cuprate PrBaCuO, the Pr cations
order antiferromagnetically at 17 K in zero field. Through a combination of
magnetic susceptibility, torque magnetometry, specific heat and interchain
transport measurements, the anisotropic temperature-magnetic field phase
diagram associated with this ordering has been mapped out. A low-temperature
spin-flop transition in the Pr sub-lattice is found to occur at the same
magnetic field strength and orientation as a dimensional crossover in the
ground state of the metallic CuO chains. This coincidence suggests that the
spin reorientation is driven by a change in the anisotropic
Rudermann-Kittel-Kasuya-Yosida (RKKY) interaction induced by a corresponding
change in effective dimensionality of the conduction electrons.Comment: 8 pages, 8 figure
Fragile three-dimensionality in the quasi-one-dimensional cuprate PrBa_2Cu_4O_8
In this article we report on the experimental realization of dimensional
crossover phenomena in the chain compound PrBaCuO using
temperature, high magnetic fields and disorder as independent tuning
parameters. In purer crystals of PrBaCuO, a highly anisotropic
three-dimensional Fermi-liquid state develops at low temperatures. This
metallic state is extremely susceptible to disorder however and localization
rapidly sets in. We show, through quantitative comparison of the relevant
energy scales, that this metal/insulator crossover occurs precisely when the
scattering rate within the chain exceeds the interchain hopping rate(s), i.e.
once carriers become confined to a single conducting element.Comment: 12 pages, 5 figures, published at
http://www.iop.org/EJ/article/1367-2630/8/9/172/njp6_9_172.htm
Angle Dependent Magnetoresistance of the Layered Organic Superconductor \kappa-(ET)2Cu(NCS)2: Simulation and Experiment
The angle-dependences of the magnetoresistance of two different isotopic
substitutions (deuterated and undeuterated) of the layered organic
superconductor \kappa-(ET)2Cu(NCS)2 are presented. The angle dependent
magnetoresistance oscillations (AMRO) arising from the quasi-one-dimensional
(Q1D) and quasi-two-dimensional (Q2D) Fermi surfaces in this material are often
confused. By using the Boltzman transport equation extensive simulations of the
AMRO are made that reveal the subtle differences between the different species
of oscillation. No significant differences are observed in the electronic
parameters derived from quantum oscillations and AMRO for the two isotopic
substitutions. The interlayer transfer integrals are determined for both
isotopic substitutions and a slight difference is observed which may account
for the negative isotope effect previously reported [1]. The success of the
semi-classical simulations suggests that non-Fermi liquid effects are not
required to explain the interlayer-transport in this system.Comment: 15 pages, 16 figure
Violation of the isotropic- approximation in overdoped La_{2-x}Sr_xCuO_4
Magnetotransport measurements on the overdoped cuprate La_{1.7}Sr_{0.3}CuO_4
are fitted using the Ong construction and band parameters inferred from
angle-resolved photoemission. Within a band picture, the low temperature Hall
data can only be fitted satisfactorily by invoking strong basal-plane
anisotropy in the mean-free-path . This violation of the isotropic-
approximation supports a picture of dominant small-angle elastic scattering in
cuprates due to out-of-plane substitutional disorder. We show that both band
anisotropy and anisotropy in the elastic scattering channel strongly
renormalize the Hall coefficient in overdoped La_{2-x}Sr_xCuO_4 over a wide
doping and temperature range.Comment: 4 pages, 4 figure
A Flexible Enterprise Needs an Adaptable eBusiness Architecture in Order to Satisfy Naturally Evolving Requirements
Standards for exchange of purchasing information, such as ANSI X-12 for EDI, have been used by large industries (e.g. retail and auto) for almost 30 years. Newer web-based tools and new standards hold the promise of reduced cost and wider applicability. For many small to medium sized enterprises, the cost and rigidity of existing tools out weight the prospective gains, which must be amortised over comparatively few transactions. In this paper, we describe the development of an N-tiered, object-oriented, architecture for interacting with suppliers based on emerging web tools. We explore the ways in which the project was required to adapt to existing purchasing systems and the ways that the project evolved during its development. We identify patterns in the inevitable evolution of requirements during the implementation, and we describe the ways that the architecture facilitated the satisfaction of these changing requirements. By analysing the major “transition points” during the development, we attempt to document the fundamental nature of evolving requirements and the need to explicitly reflect them in adaptable e-business architectures
Possible co-existence of local itinerancy and global localization in a quasi-one-dimensional conductor
In the chain compound PrBaCuO localization appears simultaneously
with a dimensional crossover in the electronic ground state when the scattering
rate in the chains exceeds the hopping rate between the chains. Here we report
the discovery of a large, transverse magnetoresistance in PrBaCuO
in the localized regime. This result suggests a novel form of localization
whereby electrons retain their metallic (quasi-one-dimensional) character over
a microscopic length scale despite the fact that macroscopically, they exhibit
localized (one-dimensional) behavior.Comment: 4 pages, 4 Figure
Irradiation-induced confinement in a quasi-one-dimensional metal
The anisotropic resistivity of PrBaCuO has been measured as a
function of electron irradiation fluence. Localization effects are observed for
extremely small amounts of disorder corresponding to electron mean-free-paths
of order 100 unit cells. Estimates of the localization corrections suggest that
this anomalous localization threshold heralds a crossover to a ground state
with pronounced one-dimensional character in which conduction electrons become
confined to a small cluster of chains.Comment: 4 pages, 4 figure
High-Field Pauli-Limiting Behavior and Strongly Enhanced Upper Critical Magnetic Fields near the Transition Temperature of an Arsenic-Deficient LaO_0.9F_0.1FeAs_(1-\delta) Superconductor
We report upper critical field B_c2(T) data for disordered
(arsenic-deficient) LaO_0.9F_0.1FeAs_(1-delta) in a wide temperature and
magnetic field range up to 47 T. Because of the large linear slope of Bc2 about
-5.4 T/K to -6.6 T/K near Tc = 28.5 K the T-dependence of the in-plane Bc2(T)
shows a flattening near 23 K above 30 T which points to Pauli-limited behavior
with Bc2(0) about 63-68 T. Our results are discussed in terms of disorder
effects within conventional and unconventional superconducting pairings.Comment: Change of the title as suggested by the Editors, one author added,
typos corrected, references updated, final published versio
Comparison of the Fermi-surface topologies of kappa-(BEDT-TTF)_2 Cu(NCS)_2 and its deuterated analogue
We have measured details of the quasi one-dimensional Fermi-surface sections
in the organic superconductor kappa-(BEDT-TTF)_2 Cu(NCS)_2 and its deuterated
analogue using angle-dependent millimetre-wave techniques. There are
significant differences in the corrugations of the Fermi surfaces in the
deuterated and undeuterated salts. We suggest that this is important in
understanding the inverse isotope effect, where the superconducting transition
temperature rises on deuteration. The data support models for superconductivity
which invoke electron-electron interactions depending on the topological
properties of the Fermi surface
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